鴻研報告:2020年材料領域Nature&Science大盤點,年度最能發文章的材料它是誰?

2021-02-25 材料人
Inverse transition of labyrinthine domain patterns in ferroelectric thin films
Localization and delocalization of light in photonic moiré lattices

Strain engineering and epitaxial stabilization of halide perovskites

Proton-assisted growth of ultra-flat graphene films

Synthesis and properties of free-standing monolayer amorphous carbon

Single-chain heteropolymers transport protons selectively and rapidly

Direct thermal neutron detection by the 2D semiconductor 6LiInP2Se6
Transparent ferroelectric crystals with ultrahigh piezoelectricity
Design and synthesis of multigrain nanocrystals via geometric misfit strain

Classification with a disordered dopant-atom network in silicon

Conversion of non-van der Waals solids to 2D transition-metal chalcogenides

Shubin Yang/Pulickel M. AjayanAntagonistic cooperativity between crystal growth modifiers

Jeffrey D.Rimer/Peter G. VekilovRedox-switchable carboranes for uranium capture and release

Gram-scale bottom-up flash graphene synthesis

Rouzbeh Shahsavari/Boris I. Yakobson/James M. TourHeterogeneous integration of single-crystalline complex-oxide membranes

Chang-Beom Eom/Jeehwan KimSpin current from sub-terahertz-generated antiferromagnetic magnons
Quantum crystal structure in the 250-kelvin superconducting lanthanum hydrideUniversity of the Basque Country
Li metal deposition and stripping in a solid-state battery via Coble creep
A droplet-based electricity generator with high instantaneous power density
Zhong Lin Wang/Xiao Cheng Zeng/Zuankai WangOn-device lead sequestration for perovskite solar cells
Wafer-scale single-crystal hexagonal boron nitride monolayers on Cu (111)

Boris I. Yakobson/Wen-Hao Chang/Lain-Jong LiSpontaneous gyrotropic electronic order in a transition-metal dichalcogenide

Pablo Jarillo-Herrero/Nuh GedikStrain-hardening and suppression of shear-banding in rejuvenated bulk metallic glass

High-pressure strengthening in ultrafine-grained metals

Ultrafast machine vision with 2D material neural network image sensors

Lukas Mennel/Thomas MuellerSingle-particle spectroscopy for functional nanomaterials

Jiajia Zhou/Alexey I. Chizhik/Steven Chu/Dayong JinTunable correlated Chern insulator and ferromagnetism in a moiré superlattice

David Goldhaber-Gordon/Yuanbo Zhang/Feng WangStrange-metal behaviour in a pure ferromagnetic Kondo lattice

Michael Smidman/Piers Coleman/Huiqiu YuanCoherent electrical control of a single high-spin nucleus in siliconSchool of Electrical Engineering and Telecommunications

In situ NMR metrology reveals reaction mechanisms in redox flow batteries

Limits on gas impermeability of graphene

Observations of grain-boundary phase transformations in an elemental metal

Timofey Frolov/Gerhard Dehm/Christian H. LiebscherAutomated radial synthesis of organic molecules

Simulation of Hubbard model physics in

WSe2/WS2 moiré superlattices



Mott and generalized Wigner crystal states in WSe2/WS2 moiré superlattices

General synthesis of two-dimensional van der Waals heterostructure arrays

Xidong Duan/Xiangfeng DuanA mechanism of ferritin crystallization revealed by cryo-STEM tomography

Chiral superconductivity in heavy-fermion metal UTe2
Collisional cooling of ultracold molecules

Direct-bandgap emission from hexagonal Ge and SiGe alloys

Control and single-shot readout of an ion embedded in a nanophotonic cavity

Layered nanocomposites by shear-flow-induced alignment of nanosheets

Performance-limiting nanoscale trap clusters at grain junctions in halide perovskites

Keshav M. Dani/Samuel D. StranksStrongly correlated electrons and hybrid excitons in a moiré heterostructure

Yuya Shimazaki/Ataç ImamoğluNon-volatile electric control of spin–charge conversion in a SrTiO3 Rashba system

Manuel Bibes/Jean-Philippe AttanéEnhanced ferroelectricity in ultrathin films grown directly on silicon
Suraj S. Cheema/Sayeef SalahuddinElectrical manipulation of a topological antiferromagnetic state
Two-dimensional halide perovskite lateral epitaxial heterostructures

Brett M. Savoie1/Yi Yu/Letian DouIron-based binary ferromagnets for transverse thermoelectric conversion

Engineering covalently bonded 2D layered materials by self-intercalation

Xin Luo/Stephen J.Pennycook/Kian Ping LohAccelerated discovery of CO2 electrocatalysts using active machine learnin
Zachary Ulissi/Edward H. SargentMapping the twist-angle disorder and Landau levels in magic-angle graphene
P.Jarillo-Herrero/E. ZeldovPreparation of cyclohexene isotopologues and stereoisotopomers from benzene

Short-range order and its impact on the CrCoNi medium-entropy alloy

A biomimetic eye with a hemispherical perovskite nanowire array retina

Spectroscopy of short-lived radioactive molecules

R. F. Garcia Ruiz1/R. BergerCascade of electronic transitions in magic-angle twisted bilayer graphene

Self-templating assembly of soft microparticles into complex tessellations

Fabio Grillo/Miguel Angel Fernandez-Rodriguez/Lucio IsaLeveraging excited-state coherence for synthetic control of ultrafast dynamics

Topological polaritons and photonic magic angles in twisted α-MoO3 bilayers

Qiaoliang Bao/Cheng-Wei Qiu/Andrea AlùCascade of phase transitions and Dirac revivals in magic-angle graphene

P. Jarillo-Herrero/S.IlaniLate-stage oxidative C(sp3)–H methylation

Confinement of atomically defined metal halide sheets in a metal–organic framework

Superstructure control of first-cycle voltage hysteresis in oxygen-redox cathodes

A general carbonyl alkylative amination for tertiary amine synthesis

Molecular tuning of CO2-to-ethylene conversion
Theodor Agapie/Jonas C. Peters/Edward H. SargentA map of the amine–carboxylic acid coupling system

Synthesis of rare sugar isomers through site-selective epimerization

Lactonization as a general route to β-C(sp3)–H functionalization

Pascal conductance series in ballistic one-dimensional LaAlO3/SrTiO3 channels

Megan Briggeman/Jeremy LevyDry reforming of methane by stable Ni-Mo nanocatalysts on single-crystalline MgO
Flux-induced topological superconductivity in full-shell nanowires
R. M. Lutchyn/C. M. MarcusHydrophobic zeolite modification for in situ peroxide formation in methane oxidation to methanol
Liang Wang/Feng-Shou XiaoRealization of the kagome spin ice state in a frustrated intermetallic compound

Kan Zhao/Philipp GegenwartHighly active cationic cobalt(II) hydroformylation catalysts

Atomic manipulation of the gap in Bi2Sr2CaCu2O8+x

Evidence for dispersing 1D Majorana channels in an iron-based superconductor

Evidence for an edge supercurrent in the Weyl superconductor MoTe2

Ferromagnetic order beyond the superconducting dome in a cuprate superconductor

Nearly quantized conductance plateau of vortex zero mode in an iron-based superconductor

Yu-Yang Zhang/Hong Ding/Hong-Jun GaoCritical differences in 3D atomic structure of individual ligand-protected nanocrystals in solution

Peter Ercius/Hans Elmlund/Jungwon Parkkinetic pathways of ionic transport in fast-charging lithium titanateBrookhaven National Laboratory
Absence of evidence for chiral Majorana modes in quantum anomalous Hall-superconductor devices

Moses H. W. Chan1/Nitin Samarth/Cui-Zu ChangOriented attachment induces fivefold twins by forming and decomposing high-energy grain boundariesPacific Northwest National Laboratory

Quantum anomalous Hall effect in intrinsic magnetic topological insulator MnBi2Te4
Jing Wang1/Xian Hui Chen/Yuanbo ZhangHelical quantum hall phase in graphene on SrTiO3
Extreme tensile strain states in La0.7Ca0.3MnO3 membranes

Visualizing H2O molecules reacting at TiO2 active sites with transmission electron microscopy

Ze Zhang/Jakob B. Wagner/Yi Gao/Yong WangCrystal symmetry determination in electron diffraction using machine learning

CO2 electrolysis to multicarbon products at activities greater than 1 A/cm2

David Sinton/Edward H. SargentGenetically targeted chemical assembly of functional materials in living cells, tissues, and animals

Zhenan Bao/Karl DeisserothIntrinsic quantized anomalous Hall effect in a moiré heterostructure

Self-induced spin glass state in elemental and crystalline neodymium

Daniel Wegner/Alexander A. KhajetooriansControlling interdependent meso-nanosecond dynamics and defect generation in metal 3D printingLawrence Livermore National Laboratory

Control of zeolite pore interior for chemoselective alkyne/olefin separations

Ionoelastomer junctions between polymer networks of fixed anions and cations

Zhigang Suo/Ryan C. HaywardRatcheting quasi-ballistic electrons in silicon geometric diodes at room temperature

Total synthesis of the complex taxane diterpene canataxpropellane

Nitromethane as a nitrogen donor in Schmidt-type formation of amides and nitriles

Total synthesis reveals atypical atropisomerism in a small-molecule natural product, tryptorubin A

Observation of hydrogen trapping at dislocations, grain boundaries, and precipitates

Hongzhou Lu/Julie M. CairneyUltrahigh-field 67Zn NMR reveals short-range disorder in zeolitic imidazolate framework glasses

Sabyasachi Sen/Yuanzheng YueRational construction of a scalable heterostructured nanorod megalibrary

Fluorination of arylboronic esters enabled by bismuth redox catalysis

One-dimensional van der Waals heterostructures

Rong Xiang/Shigeo MaruyamaRoom temperature magnetoelectric coupling in a molecular ferroelectric ytterbium complex
Observation of an isomerizing double-well quantum system in the condensed phase

Efficient tandem solar cells with solution-processed perovskite on textured crystalline silicon

Stefaan De Wolf/Edward H. SargentCatalyst-controlled doubly enantioconvergent coupling of racemic alkyl nucleophiles and electrophiles

Subwavelength dielectric resonators for nonlinear nanophotonics

Hong-Gyu Park/Yuri KivsharSubterahertz spin pumping from an insulating antiferromagnet
Topological structure and dynamics of three-dimensional active nematics

Daniel A. Beller/Zvonimir DogicObservation of the fastest chemical processes in the radiolysis of water

Z.-H. Loh/R. Santra/L. YoungGiant thermopower of ionic gelatin near room temperature

Triple-halide wide–band gap perovskites with suppressed phase segregation for efficient tandems

Jixian Xu/Michael D. McGeheeNa+-gated water-conducting nanochannels for boosting CO2 conversion to liquid fuelsUltrahigh thermal conductivity in isotope enriched cubic boron nitride

Bai Song/David Broido/Gang ChenBiocatalytic synthesis of planar chiral macrocycles

DNA-directed nanofabrication of high-performance carbon nanotube field-effect transistors

Precise pitch-scaling of carbon nanotube arrays within three-dimensional DNA nanotrenches

Photoelectron spectra of alkali metal–ammonia microjets: From blue electrolyte to bronze metalCzech Academy of Sciences

Ondrej Marsalek/Bernd Winter/Stephen E. Bradforth/Pavel JungwirthTwisted bulk-boundary correspondence of fragile topology

Experimental characterization of fragile topology in an acoustic metamaterial

A general method to synthesize and sinter bulk ceramics in seconds

Xiaoyu (Rayne) Zheng/Jian Luo/Yifei Mo/Liangbing HuEmergence of complexity in hierarchically organized chiral particles

André F. de Moura/Nicholas A. KotovPhonon hydrodynamics and ultrahigh–room-temperature thermal conductivity in thin graphite

Balancing volumetric and gravimetric uptake in highly porous materials for clean energy

Entanglement-based single-shot detection of a single magnon with a superconducting qubit

Resolving spatial and energetic distributions of trap states in metal halide perovskite solar cells
Enantioselective remote C–H activation directed by a chiral cation

Disassembling 2D van der Waals crystals into macroscopic monolayers and reassembling into artificial lattices

Efficient, stable silicon tandem cells enabled by anion-engineered wide-bandgap perovskites
Jin Young Kim/Kai Zhu/Dong Hoe Kim/Byungha ShinFrequency-comb spectroscopy on pure quantum states of a single molecular ion

Water-promoted interfacial pathways in methane oxidation to methanol on a CeO2-Cu2O catalystBrookhaven National Laboratory

Ping Liu/José A. Rodriguez/Sanjaya D. SenanayakeA dual light-driven palladium catalyst:Breaking the barriers in carbonylation reactions

Aligned, high-density semiconducting carbon nanotube arrays for high-performance electronics

Zhiyong Zhang/Lian-Mao PengDiverse functionalization of strong alkyl C–H bonds by undirected borylation

Three-dimensional cross-nanowire networks recover full terahertz state
Synthesis of proteins by automated flow chemistry

Iridium-catalyzed acid-assisted asymmetric hydrogenation of oximes to hydroxylamines

Self-assembly of a layered two-dimensional molecularly woven fabric

Topological superconductivity in a van der Waals heterostructure
Shawulienu Kezilebieke/Teemu Ojanen/Peter LiljerothStrongly correlated Chern insulators in magic-angle twisted bilayer graphene
Ultrafast structural changes within a photosynthetic reaction centre

Metallaphotoredox aryl and alkyl radiomethylation for PET ligand discovery

Lanthanide-doped inorganic nanoparticles turn molecular triplet excitons bright
Renren Deng/Xiaogang Liu/Akshay RaoSpin-enhanced nanodiamond biosensing for ultrasensitive diagnosticsBenjamin S. Miller/Rachel A. McKendryUnconventional ferroelectricity in moiré heterostructuresQiong Ma/Pablo Jarillo-HerreroKey role of chemistry versus bias in electrocatalytic oxygen evolution

Detre Teschner/Travis E. JonesCorrelated insulating states at fractional fillings of moiré superlattices
Yang Xu/Veit Elser/ Kin Fai Mak/Jie ShanAnatomy of cage formation in a two-dimensional glass-forming liquid

Bo Li/Walter Kob/Steve GranickCatalytic asymmetric addition of an amine N–H bond across internal alkenes

Metal-free photoinduced C(sp3)–H borylation of alkanes

Adam Noble/Varinder K. AggarwalEfficient epoxidation over dinuclear sites in titanium silicalite-1
High-throughput calculations of magnetic topological materialsSurface coordination layer passivates oxidation of copper

Gang Fu/Ying Jiang/Nanfeng ZhengRoom-temperature superconductivity in a carbonaceous sulfur hydride

Efficient and stable blue quantum dot light-emitting diode
An enzymatic Alder-ene reaction

 Jiahai Zhou/K. N. Houk/Yi TangConcentric liquid reactors for chemical synthesis and separation

Graphene-based Josephson junction microwave bolometer
Fractional antiferromagnetic skyrmion lattice induced by anisotropic couplings

Near-perfect photon utilization in an air-bridge thermophotovoltaic cell
Andrej Lenert/Stephen R. ForrestPlasmonic enhancement of stability and brightness in organic light-emitting devices

Reverse and forward engineering of Drosophila corneal nanocoatings
Rare-earth–platinum alloy nanoparticles in mesoporous zeolite for catalysis
Filling metal–organic framework mesopores with TiO2 for CO2 photoreduction
Osamu Terasaki/Ling Zan/Hexiang DengStable room-temperature continuous-wave lasing in quasi-2D perovskite films

Chuanjiang Qin/Chihaya AdachiA disordered rock salt anode for fast-charging lithium-ion batteries
Jun Lu/Huolin L. Xin/Shyue Ping Ong/Ping LiuTying different knots in a molecular strand

Intercepting fleeting cyclic allenes with asymmetric nickel catalysis

Observation of superconducting diode effect

Liquid–liquid transition and critical point in sulfur

Additive manufacturing of silica aerogels

Shanyu Zhao/Wim J. MalfaitPiezoelectric and pyroelectric effects induced by interface polar symmetry

Ming-Min Yang/Marin AlexeCoupling dinitrogen and hydrocarbons through aryl migration

Evidence of flat bands and correlated states in buckled graphene superlattices
Yuhang Jiang/Eva Y. AndreiElectronic phase separation in multilayer rhombohedral graphite
A photochemical dehydrogenative strategy for aniline synthesis

A fabrication process for flexible single-crystal perovskite devices

Deep strong light–matter coupling in plasmonic nanoparticle crystals
Imaging viscous flow of the Dirac fluid in graphene
Amir Yacoby/Ronald L. WalsworthQuantum-limit Chern topological magnetism in TbMn6Sn6
Jia-Xin Yin/Shuang Jia/M. Zahid HasanCleavable comonomers enable degradable, recyclable thermoset plastics

Coherent many-body exciton in van der Waals antiferromagnet NiPS3
Ke-Jin Zhou/Young-Woo Son/Jae Hoon Kim/Hyeonsik Cheong/Je-Geun ParkSelf-assembled poly-catenanes from supramolecular toroidal building blocks
Monolithic piezoelectric control of soliton microcombs

Sunil A. Bhave/Tobias J. KippenbergSuperconductivity in metallic twisted bilayer graphene stabilized by WSe2
Vacancy-enabled N2 activation for ammonia synthesis on an Ni-loaded catalyst
Masaaki Kitano/Hideo HosonoA subradiant optical mirror formed by a single structured atomic layer

Compression of curium pyrrolidine-dithiocarbamate enhances covalency
Manfred Speldrich/Eva Zurek/Jochen Autschbach/Thomas E. Albrecht-SchönzartTunable spin-polarized correlated states in twisted double bilayer graphene
Untying the insulating and superconducting orders in magic-angle grapheneChemical gradients in human enamel crystallites

Tailored quinones support high-turnover Pd catalysts for oxidative C–H arylation with O2
Monolithic perovskite/silicon tandem solar cell with >29% efficiency by enhanced hole extraction
Reversible planar gliding and microcracking in a single-crystalline Ni-rich cathode
Constrained minimal-interface structures in polycrystalline copper with extremely fine grains

Nano-acoustic resonator with ultralong phonon lifetime
Prebiotic synthesis of cysteine peptides that catalyze peptide ligation in neutral water
Large-area low-noise flexible organic photodiodes for detecting faint visible light

Canek Fuentes-Hernandez/Bernard KippelenAtomic-scale microstructure of metal halide perovskite

Peter D. Nellist/Laura M. HerzMetal-organic magnets with large coercivity and ordering temperatures up to 242°C

Itziar Oyarzabal/Rodolphe CléracCdPS3 nanosheets-based membrane with high proton conductivity enabled by Cd vacancies

design of higher valency in covalent organic frameworks

Polyethylene upcycling to long-chain alkylaromatics by tandem hydrogenolysis/aromatization
Metasurface-driven OLED displays beyond 10,000 pixels per inch

Won-Jae Joo/Mark L. BrongersmaSupertwisted spirals of layered materials enabled by growth on non-Euclidean surfaces
Cartilage-inspired, lipid-based boundary-lubricated hydrogels

Ronit Goldberg1/Jacob KleinThermosensitive crystallization–boosted liquid thermocells for low-grade heat harvesting

Structural and spectroscopic characterization of an Fe(VI) bis(imido) complex

Recent advances in solid oxide cell technology for electrolysis
Black phosphorus composites with engineered interfaces for high-rate high-capacity lithium storage
Hengxing Ji/Xiangfeng DuanElectro-inductive effect: Electrodes as functional groups with tunable electronic properties

Sang Woo Han/Mu-Hyun BaikClean 2D superconductivity in a bulk van der Waals superlattice
Vapor-assisted deposition of highly efficient, stable black-phase FAPbI3 perovskite solar cells
Yiqiang Zhan/Lirong Zheng/Anders Hagfeldt/Michael GrätzelMultiplicity of dislocation pathways in a refractory multiprincipal element alloy

A universal system for digitization and automatic execution of the chemical synthesis literature

Impact of strain relaxation on performance of a-formamidinium lead iodide perovskite solar cells
Inducing metallicity in graphene nanoribbons via zero-mode superlattices
Steven G. Louie/Felix R. Fischer/Michael F. CrommieStable perovskite solar cells with efficiency exceeding 24.8% and 0.3-V voltage loss
Sang Kyu Kwak/Dong Suk Kim/Changduk YangReversible structural transformations in supercooled liquid water from 135 to 245 K

Bruce D. Kay/Greg A. KimmelFollowing the microscopic pathway to adsorption through chemisorption and physisorption wells

Self-limiting directional nanoparticle bonding governed by reaction stoichiometry

Eugenia Kumacheva/Zhihong NieAccelerating water dissociation in bipolar membranes and for electrocatalysis
Sebastian Z. Oener/Shannon W. BoettcherSuper-durable ultralong carbon nanotubes

Static to inducibly dynamic stereocontrol: The convergent use of racemic β-substituted ketones

David W. C. MacMillan/Todd K. HysterCovalent surface modifications and superconductivity of two-dimensional metal carbide MXenes
Asymmetric remote C–H borylation of aliphatic amides and esters with a modular iridium catalyst
Shaping colloidal bananas to reveal biaxial, splay-bend nematic, and smectic phases

Iron-based superelastic alloys with near-constant critical stress temperature dependence

A molecular mediator for reductive concerted proton-electron transfers via electrocatalysis

Observation of small Fermi pockets protected by clean CuO2 sheets of a high-Tc superconductor

Kazuyasu Tokiwa/Takeshi KondoDivergent synthesis of complex diterpenes through a hybrid oxidative approach

A short de novo synthesis of nucleoside analogs


Sequencing of metals in multivariate metal organic frameworks

Chemical vapor deposition of layered two-dimensional MoSi2N4 materials
Direct reversible decarboxylation from stable organic acids in dimethylformamide solution

Rational synthesis of atomically precise graphene nanoribbons directly on metal oxide surfaces
An-Ping Li/Konstantin AmsharovExceptional plasticity in the bulk single-crystalline van der Waals semiconductor InSe

Lidong Chen/Jian He/Xun ShiBoosted molecular mobility during common chemical reactions

Anomalous absorption of electromagnetic waves by 2D transition metal carbonitride Ti3CNTx (MXene)

Yury Gogotsi/Chong Min KooUltrahigh-strength and ductile superlattice alloys with nanoscale disordered interfaces
Cooperative carbon capture and steam regeneration with tetraamine-appended metal–organic frameworks

N-Aryl–linked spirocyclic polymers for membrane separations of complex hydrocarbon mixtures

Ryan P. Lively/M. G. FinnBoron-enabled geometric isomerization of alkenes via selective energy-transfer catalysis

John J. Molloy/Ryan GilmourGiant piezoelectricity in oxide thin films with nanopillar structure
Observation and control of maximal Chern numbers in a chiral topological semimetal

Niels B. M. Schröter/Claudia FelserUltrahigh capacitive energy density in ion-bombarded relaxor ferroelectric films
C(sp3)–H functionalizations of light hydrocarbons using decatungstate photocatalysis in flow
A piperidinium salt stabilizes efficient metal-halide perovskite solar cells
Yen-Hung Lin/Henry J. Snaith

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